Greek Language Kits - The Media & Design Center offers a variety of Greek Language Kits to help facilitate in learning the Greek Language.
Greek Dictionaries - UNC Libraries have several Greek Language Dictionaries for checkout. Such as the Oxford Greek-English Learner's Dictionary.
Greek Customs - When showing interest in learning a different language, it's important to also learn some of the customs of native speakers. Many resources can found in the library and online. For example, Hellenism.net and everyculture.com.
Greek Movies - The MDC also has many movies in Greek to help facilitate learning in all your language pursuits. Here are just few of the titles available.